Thermodiffusion of the tetrahydronaphthalene and dodecane mixture under high pressure and in porous medium

Cédric Giraudet; Fabrizio Croccolo; Guillaume Galliero; Gilles Pijaudier-Cabot; Stefan Van Vaerenbergh; M. Ziad Saghir; François Montel; Henri Bataller

doi:10.1016/j.crme.2013.01.007

Thermodiffusion of the tetrahydronaphthalene and dodecane mixture under high pressure and in porous medium

Cédric Giraudet ¹; Fabrizio Croccolo ²; Guillaume Galliero ¹; Gilles Pijaudier-Cabot ¹; Stefan Van Vaerenbergh ³; M. Ziad Saghir ⁴; François Montel ⁵; Henri Bataller ¹

¹ Laboratoire des Fluides Complexes et leurs Réservoirs, UMR 5150, Université de Pau et des Pays de lʼAdour, BP 1155, 64013 Pau cedex, France
² Physics Department, University of Fribourg, chemin du Musée 3, 1700 Fribourg, Switzerland
³ Microgravity Research Center, Université Libre de Bruxelles, CP165/62, 1150 Bruxelles, Belgium
⁴ Ryerson University, 350 Victoria St, Toronto, ONT, M5B 2K3, Canada
⁵ Total SA, avenue Larribau, 64018 Pau cedex, France

Comptes Rendus. Mécanique, 10th International Meeting on Thermodiffusion, Volume 341 (2013) no. 4-5, pp. 340-347.

Abstract

A thermodiffusion cell is used in order to perform Soret experiments on binary mixtures at high pressure and in the presence of a porous medium. The cell is validated at atmospheric pressure with toluene/hexane and the tetrahydronaphthalene/dodecane mixtures. The mass separation follows a diffusive behaviour when the cell is filled with a porous medium. At least three times the relaxation time is needed to have a good estimation of the Soret coefficients. From the transient state of the mass separation and using accepted values of the diffusion coefficient, the tortuosity of the porous medium was evaluated, too. Finally, experiments at high pressure were performed with the tetrahydronaphthalene/dodecane system. In these experiments, decreases of the Soret coefficient and of the tortuosity of the porous medium were measured as a function of the pressure.

Published online: 2013-02-20

DOI: 10.1016/j.crme.2013.01.007

Keywords: Thermodiffusion cell, Porous medium, Tortuosity, Molecular diffusion coefficient, Soret coefficient, High pressure

Author's affiliations:

Cédric Giraudet ¹; Fabrizio Croccolo ²; Guillaume Galliero ¹; Gilles Pijaudier-Cabot ¹; Stefan Van Vaerenbergh ³; M. Ziad Saghir ⁴; François Montel ⁵; Henri Bataller ¹

¹ Laboratoire des Fluides Complexes et leurs Réservoirs, UMR 5150, Université de Pau et des Pays de lʼAdour, BP 1155, 64013 Pau cedex, France
² Physics Department, University of Fribourg, chemin du Musée 3, 1700 Fribourg, Switzerland
³ Microgravity Research Center, Université Libre de Bruxelles, CP165/62, 1150 Bruxelles, Belgium
⁴ Ryerson University, 350 Victoria St, Toronto, ONT, M5B 2K3, Canada
⁵ Total SA, avenue Larribau, 64018 Pau cedex, France

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     author = {C\'edric Giraudet and Fabrizio Croccolo and Guillaume Galliero and Gilles Pijaudier-Cabot and Stefan Van Vaerenbergh and M. Ziad Saghir and Fran\c{c}ois Montel and Henri Bataller},
     title = {Thermodiffusion of the tetrahydronaphthalene and dodecane mixture under high pressure and in porous medium},
     journal = {Comptes Rendus. M\'ecanique},
     pages = {340--347},
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     year = {2013},
     doi = {10.1016/j.crme.2013.01.007},
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%A Cédric Giraudet
%A Fabrizio Croccolo
%A Guillaume Galliero
%A Gilles Pijaudier-Cabot
%A Stefan Van Vaerenbergh
%A M. Ziad Saghir
%A François Montel
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Cédric Giraudet; Fabrizio Croccolo; Guillaume Galliero; Gilles Pijaudier-Cabot; Stefan Van Vaerenbergh; M. Ziad Saghir; François Montel; Henri Bataller. Thermodiffusion of the tetrahydronaphthalene and dodecane mixture under high pressure and in porous medium. Comptes Rendus. Mécanique, 10th International Meeting on Thermodiffusion, Volume 341 (2013) no. 4-5, pp. 340-347. doi : 10.1016/j.crme.2013.01.007. https://comptes-rendus.academie-sciences.fr/mecanique/articles/10.1016/j.crme.2013.01.007/

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