Comptes Rendus
no. 3
Agrégats comme précurseurs des nano-objets/Clusters as precursors of nano-objects
Mass selected cluster deposition in strongly or weakly interacting media
[Déposition d'agrégats triés en taille dans des milieux avec de fortes ou faibles interactions]
Wolfgang Harbich1  ; Christian Félix1
1 Institut de physique des nanostructures, Faculté des sciences de base, École polytechnique fédérale, CH-1015 Lausanne, Switzerland
Comptes Rendus. Physique, Volume 3 (2002) no. 3, pp. 289-300.

La déposition d'agrégats sélectionnés en taille est discutée en rapport avec trois questions : quelle est l'inégrité des agrégats après la déposition, quelle est leur uniformité en terme de taille et d'isomérisation et finalement quelle est l'influence du support ? La réponse à ces questions dépendra de la force de l'interaction entre l'agrégat et le milieu dans lequel il se trouve. Nous avons choisi deux cas extrêmes : les gaz rares inertes d'un côté et des surfaces métalliques de l'autre. Trois exemples sont discutés : Des études des spectroscopie Raman ainsi que des mesures de microscopie tunnel donnent des informations de structure géométrique sur les agrégats déposés, alors que d'autres spectroscopies optiques (absoption et fluorescence) livrent des informations sur leur structure électronique.

Mass selected cluster deposition is discussed with respect to three questions: what is the integrity of the clusters after deposition; are they uniform in terms of size and isomerisation; and finally what is the influence of the support on the clusters? The answer to these questions will depend on the strength of cluster media interaction and we have chosen two extreme cases the inert rare gases on one hand and metal surfaces on the other. Three examples are given: Raman studies as well as low-temperature STM give structural information on the deposited clusters, while other optical spectroscopies (absorption and fluorescence) yield information on the electronic structure of the clusters.

Reçu le :
Accepté le :
Publié le :
DOI : 10.1016/S1631-0705(02)01320-8
Keywords: cluster deposition, softlanding, geometrical structure, electronic structure
Mots-clés : deposition d'agrégats, structure geométrique, structure electronique

Wolfgang Harbich 1 ; Christian Félix 1

1 Institut de physique des nanostructures, Faculté des sciences de base, École polytechnique fédérale, CH-1015 Lausanne, Switzerland 
@article{CRPHYS_2002__3_3_289_0,
     author = {Wolfgang Harbich and Christian F\'elix},
     title = {Mass selected cluster deposition in strongly or weakly interacting media},
     journal = {Comptes Rendus. Physique},
     pages = {289--300},
     publisher = {Elsevier},
     volume = {3},
     number = {3},
     year = {2002},
     doi = {10.1016/S1631-0705(02)01320-8},
     language = {en},
}
TY  - JOUR
AU  - Wolfgang Harbich
AU  - Christian Félix
TI  - Mass selected cluster deposition in strongly or weakly interacting media
JO  - Comptes Rendus. Physique
PY  - 2002
SP  - 289
EP  - 300
VL  - 3
IS  - 3
PB  - Elsevier
DO  - 10.1016/S1631-0705(02)01320-8
LA  - en
ID  - CRPHYS_2002__3_3_289_0
ER  - 
%0 Journal Article
%A Wolfgang Harbich
%A Christian Félix
%T Mass selected cluster deposition in strongly or weakly interacting media
%J Comptes Rendus. Physique
%D 2002
%P 289-300
%V 3
%N 3
%I Elsevier
%R 10.1016/S1631-0705(02)01320-8
%G en
%F CRPHYS_2002__3_3_289_0
Wolfgang Harbich; Christian Félix. Mass selected cluster deposition in strongly or weakly interacting media. Comptes Rendus. Physique, Volume 3 (2002) no. 3, pp. 289-300. doi : 10.1016/S1631-0705(02)01320-8. https://comptes-rendus.academie-sciences.fr/physique/articles/10.1016/S1631-0705(02)01320-8/

[1] Proccedings of ISSPIC IV, Berlin, 1984, Springer-Verlag, Berlin, Heidelberg, New York, 1984

[2] W. Schulze; H. Becker; H. Abe Chem. Phys., 35 (1978), p. 177

[3] E. Parks; B. Weiller; P. Bechthold; W. Hoffmann; G. Niemann; L. Pobo; S. Riley J. Chem. Phys., 88 (1988), p. 1622

[4] A. Sanchez; S. Abbet; U. Heiz; W.D. Schneider; H. Hakkinen; R.N. Barnett; U. Landman J. Phys. Chem. A., 103 (1999), p. 9573

[5] P. Fayet; F. Granzer; G. Hegenbart; E. Moisar; B. Pischel; L. Woste Phys. Rev. Lett., 55 (1985), p. 3002

[6] P. Fayet; L. Wöste Surf. Sci., 156 (1985), p. 134

[7] H.V. Roy; P. Fayet; F. Patthey; W.D. Schneider; B. Delley; C. Massobrio Phys. Rev. B, 49 (1994), p. 5611

[8] C. Felix; G. Vandoni; C. Massobrio; R. Monot; J. Buttet; W. Harbich Phys. Rev. B, 57 (1998), p. 4048

[9] J.T. Lau; A. Achleitner; W. Wurth Chem. Phys. Lett., 317 (2000), p. 3

[10] U. Heiz; F. Vanolli; L. Trento; W.D. Schneider Rev. Sci. Instrum., 68 (1997), p. 1986

[11] T. Leisner; C. Rosche; S. Wolf; F. Granzer; L. Woeste Surf. Rev. Lett., 3 (1996), p. 1105

[12] K.J. Boyd; A. Lapicki; M. Aizawa; S.L. Anderson Rev. Sci. Instrum., 69 (1998), p. 4106

[13] H. Jodicke; R. Schaub; A. Bhowmick; R. Monot; J. Buttet; W. Harbich Rev. Sci. Instrum., 71 (2000), p. 2818

[14] W. Harbich Collision of Clusters with Surfaces: Deposition, Surface Modifications and Scattering (K.H. Meiwes-Broer, ed.), Springer-Verlag, Berlin, 2000

[15] B. Nacer; C. Massobrio; C. Felix Phys. Rev. B, 56 (1997), p. 10590

[16] S. Fedrigo; W. Harbich; J. Beljaev; J. Buttet Chem. Phys. Lett., 211 (1993), p. 166

[17] K. Bromann; C. Felix; H. Brune; W. Harbich; R. Monot; J. Buttet; K. Kern Science, 274 (1996), p. 956

[18] S. Fedrigo; W. Harbich; J. Buttet Phys. Rev. B, 58 (1998), p. 7428

[19] B.N. Cyvin; E. Brendsdal; J. Brunvoll; S.J. Cyvin J. Mol. Struct., 352/353 (1995), p. 481

[20] V. Parasuk; J. Almlöf Chem. Phys. Lett., 184 (1991), p. 187

[21] C.J. Barbec; E.B. Anderson; B.N. Davidson; S.A. Kajihara; Q.-M. Zhang; J. Bernholc; D. Tomanek Phys. Rev. B, 46 (1992), p. 7326

[22] H.W. Kroto; K. McKay Nature, 331 (1988), p. 328

[23] A.K. Ott; G.A. Rechtsteiner; C. Felix; P. Hampe; M.F. Jarrold; R.P. Van Duyne; K. Raghavachari J. Chem. Phys., 109 (1998), p. 9652

[24] E.C. Honea; A. Ogura; D.R. Peale; C. Félix; C.A. Murray; K. Raghavachari; W.O. Sprenger; M.F. Jarrold; W.L. Brown J. Chem. Phys., 110 (1999), p. 12161

[25] A.D. Becke J. Chem. Phys., 98 (1993), p. 5648

[26] T.H.J. Dunning J. Chem. Phys., 90 (1989), p. 1007

[27] G. von Helden; M.-T. Hsu; N. Gotts; M.T. Bowers J. Phys. Chem., 97 (1993), p. 8182

[28] K.B. Shelimov; J.M. Hunter; M.F. Jarrold Int. J. Mass Spectrom. Ion Processes, 138 (1994), p. 17

[29] S.B.H. Bach; J.R. Eyler J. Chem. Phys., 92 (1990), p. 358

[30] W.A. de Heer Rev. Mod. Phys., 65 (1993), p. 611

[31] H. Parks, Private communication

[32] H. Brune Surf. Sci. Rep., 31 (1998), p. 121

[33] R. Schaub; H. Jödicke; F. Brunet; R. Monot; J. Buttet; W. Harbich Phys. Rev. Lett., 86 (2001), p. 3590

[34] U. Kreibig; M. Vollmer Optical Properties of Metal Clusters, Springer Series in Material Science, 25, Springer, Berlin, 1995

[35] J. Tiggesbaumker; L. Koller; K.H. Meiwes Broer; A. Liebsch Phys. Rev. A, 48 (1993), p. R1749

[36] W. Harbich; S. Fedrigo; J. Buttet Chem. Phys. Lett., 195 (1992), p. 5

[37] W. Harbich; S. Fedrigo; J. Buttet Z. Phys. D, 26 (1993), p. 138

[38] C. Ellert; M. Schmidt; C. Schmitt; T. Reiners; H. Haberland Phys. Rev. Lett., 75 (1995), p. 1731

[39] C. Ellert; M. Schmidt; T. Reiners; H. Haberland Z. Phys. D, 39 (1997), p. 317

[40] C. Félix; C. Sieber; W. Harbich; J. Buttet; I. Rabin; W. Schulze; G. Ertl Chem. Phys. Lett., 313 (1999), p. 105

[41] C. Félix; C. Sieber; W. Harbich; J. Buttet; I. Rabin; W. Schulze; G. Ertl Phys. Rev. Lett., 86 (2001), p. 2992

[42] I. Rabin; W. Schulze; G. Ertl J. Chem. Phys., 108 (1998), p. 5137

[43] T.P. Bigioni; R.L. Whetten; O. Dag J. Phys. Chem. B, 104 (2000), p. 6983

[44] J.P. Wilcoxon; J.E. Martin; F. Parsapour; B. Wiedenman; D.F. Kelley J. Chem. Phys., 108 (1998), p. 9137

[45] P.S. Bechthold; U. Kettler; W. Krasser Surf. Sci., 156 (1985), p. 875

[46] S. Fedrigo; W. Harbich; J. Buttet J. Chem. Phys., 99 (1993), p. 5712

[47] H. Ruppe; S. Rutz; E. Schreiber; L. Wöste Chem. Phys. Lett., 257 (1996), p. 3

[48] V.E. Bondybey; T.A. Miller Molecular Ions: Spectroscopy, Structure and Chemistry (T.A. Miller; V.E. Bondybey, eds.), North-Holland, Amsterdam, 1983

[49] M. Jacox J. Phys. Chem. Ref. Data, 27 (1998), p. 115

[50] V. Bonacic-Koutecky; V. Veyret; R. Mitric J. Chem. Phys., 115 (2001), p. 10450

[51] W. Harbich; Y. Belyaev; R. Kleiber; J. Buttet Surf. Rev. Lett., 3 (1996), p. 1147

  • Arkadiusz P. Mika; Patrick Rousseau; Alicja Domaracka; Bernd A. Huber Interaction of multiply charged ions with large free silver nanoparticles: Multielectron capture, fragmentation, and sputtering phenomena, Physical Review B, Volume 100 (2019) no. 7 | DOI:10.1103/physrevb.100.075439
  • Rudy Delaunay; Arkadiusz Mika; Alicja Domaracka; Bernd A. Huber; Patrick Rousseau Ion-collision induced molecular growth in polycyclic aromatic hydrocarbon clusters: comparison of C16H10 structural isomers, The European Physical Journal D, Volume 72 (2018) no. 9 | DOI:10.1140/epjd/e2018-90147-2
  • Detlef Schooss; Patrick Weis; Oliver Hampe; Manfred M. Kappes Determining the size-dependent structure of ligand-free gold-cluster ions, Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Volume 368 (2010) no. 1915, p. 1211 | DOI:10.1098/rsta.2009.0269
  • Albrecht Lindinger; Vlasta BonaČić-Koutecký; Roland Mitrić; David Tannor; Christiane P. Koch; Volker Engel; Thorsten M. Bernhardt; Joshua Jortner; Aldo Mirabal; Ludger Wöste Analysis and control of small isolated molecular systems, Analysis and Control of Ultrafast Photoinduced Reactions, Volume 87 (2007), p. 25 | DOI:10.1007/978-3-540-68038-3_2
  • L.K. Zang; Y.X. Wang; Z.Y. Pan; L. Zhou; T.J. Liu; J. Zhu; X.M. Jiang Ar-buffer-assisted deposition of Cu13 on Cu(111) surfaces, Surface Science, Volume 600 (2006) no. 3, p. 527 | DOI:10.1016/j.susc.2005.11.002
  • L.K. Zang; Z.Y. Pan; Y.X. Wang; Q. Wei; L. Zhou; T.J. Liu; Z.J. Li Structure character of copper clusters deposited on argon, Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Volume 228 (2005) no. 1-4, p. 16 | DOI:10.1016/j.nimb.2004.10.015
  • J. T. Lau; A. Achleitner; H.-U. Ehrke; U. Langenbuch; M. Reif; W. Wurth Ultrahigh vacuum cluster deposition source for spectroscopy with synchrotron radiation, Review of Scientific Instruments, Volume 76 (2005) no. 6 | DOI:10.1063/1.1921551
  • J. T. Lau; W. Wurth; H.-U. Ehrke; A. Achleitner Soft landing of size-selected clusters in rare gas matrices, Low Temperature Physics, Volume 29 (2003) no. 3, p. 223 | DOI:10.1063/1.1542443

Cité par 8 documents. Sources : Crossref

Commentaires - Politique