Comptes Rendus
Research article
Bubble breakup probability in turbulent flows
Comptes Rendus. Mécanique, Volume 353 (2025), pp. 1351-1364

Bubbles drive gas and chemical transfers in various industrial and geophysical contexts, in which flows are typically turbulent. As gas and chemical transfers are bubble size dependent, a robust quantification requires a prediction of bubble breakup. The most common idea, introduced independently by Kolmogorov in 1949 and Hinze in 1955, is to consider a sharp limit between breaking and non breaking bubbles, given by $\operatorname{We}_c\approx 1$, where the Weber number $\operatorname{We}$ is the ratio between inertial and capillary forces at the bubble scale. In the statistically stationary state, $\operatorname{We}_c$ sets the maximum bubble size. Yet, due to the inherent stochasticity of the flow every bubble might in reality break. In this work, we use a stochastic linear model previously developed to infer the breakup probability of bubbles in turbulence as function of both $\operatorname{We}$ and the residence time. This allows us to introduce a definition of the critical Weber number accounting for the time spent by bubbles within a turbulent region, extending the stationary description. We show that bubble breakup is a memoryless process, whose breakup rate varies exponentially with $\operatorname{We}^{-1}$. The linear model successfully reproduces experimental breakup rates from the literature. We show that the stochastic nature of bubble breakup is central when the residence time of bubbles is smaller than ten correlation times of turbulence at the bubble scale: the transition between breaking and non breaking bubbles is smooth and most bubbles can break. For large residence times, the original vision of Kolmogorov and Hinze is recovered.

Les bulles contrôlent les réactions chimiques et les transferts de gaz pour un grand nombre de situations industrielles et naturelles caractérisées, typiquement, par des écoulements turbulents. Les transferts de gaz aux interfaces et les réactions chimiques étant fonction de la taille des bulles, pour les décrire précisément il est nécessaire de connaître leur distribution de taille et en particulier de prédire leur cassure. L’idée la plus répandue, introduite indépendamment par Kolmogorov en 1949, puis Hinze en 1951, consiste à considérer une limite stricte entre bulles stables et instables, donnée par $\operatorname{We}_c \approx 1$, où le nombre de Weber, $\operatorname{We}$, est le ratio entre forces inertielles et capillaires à l’échelle de la bulle. En régime statistiquement stationnaire, $\operatorname{We}_c$ fixe une taille maximum. Or, de part le caractère intrinsèquement fluctuant de la turbulence, toutes les bulles pourraient en réalité casser. Dans ce travail, nous utilisons un modèle linéaire stochastique développé précédemment pour prédire la probabilité de cassure en fonction du $\operatorname{We}$ mais aussi du temps passé par les bulles dans l’écoulement turbulent, nommé le temps de résidence. Ceci nous permet d’introduire un $\operatorname{We}_c$ qui prend maintenant en compte le temps de résidence, étendant ainsi la vision stationnaire. Nous montrons que le processus de cassure est un processus sans mémoire, associé à des taux de cassure variant exponentiellement en $\operatorname{We}^{-1}$. Ce modèle linéaire reproduit les taux de cassure expérimentaux présents dans la littérature. Nous montrons que la nature stochastique de la cassure est centrale lorsque les temps de résidence sont inférieurs à 10 temps de corrélation de la turbulence à l’échelle de la bulle : la transition entre bulles qui cassent et qui ne cassent pas est continue et la majorité des bulles peuvent casser. En revanche, pour des temps longs, nous retrouvons la limite stricte introduite par Kolmogorov et Hinze.

Received:
Revised:
Accepted:
Published online:
DOI: 10.5802/crmeca.343
Keywords: Bubble, turbulence, breakup, stochastic model
Mots-clés : Bulle, turbulence, cassure, modèle stochastique

Aliénor Rivière  1 , 2 ; Stéphane Perrard  2

1 LFMI, School of Engineering, EPFL, Lausanne, 1000, Switzerland
2 PMMH, CNRS, ESPCI Paris, Université PSL, Sorbonne Université, Université de Paris, 75005 Paris, France
License: CC-BY 4.0
Copyrights: The authors retain unrestricted copyrights and publishing rights
@article{CRMECA_2025__353_G1_1351_0,
     author = {Ali\'enor Rivi\`ere and St\'ephane Perrard},
     title = {Bubble breakup probability in turbulent flows},
     journal = {Comptes Rendus. M\'ecanique},
     pages = {1351--1364},
     year = {2025},
     publisher = {Acad\'emie des sciences, Paris},
     volume = {353},
     doi = {10.5802/crmeca.343},
     language = {en},
}
TY  - JOUR
AU  - Aliénor Rivière
AU  - Stéphane Perrard
TI  - Bubble breakup probability in turbulent flows
JO  - Comptes Rendus. Mécanique
PY  - 2025
SP  - 1351
EP  - 1364
VL  - 353
PB  - Académie des sciences, Paris
DO  - 10.5802/crmeca.343
LA  - en
ID  - CRMECA_2025__353_G1_1351_0
ER  - 
%0 Journal Article
%A Aliénor Rivière
%A Stéphane Perrard
%T Bubble breakup probability in turbulent flows
%J Comptes Rendus. Mécanique
%D 2025
%P 1351-1364
%V 353
%I Académie des sciences, Paris
%R 10.5802/crmeca.343
%G en
%F CRMECA_2025__353_G1_1351_0
Aliénor Rivière; Stéphane Perrard. Bubble breakup probability in turbulent flows. Comptes Rendus. Mécanique, Volume 353 (2025), pp. 1351-1364. doi: 10.5802/crmeca.343

[1] Andreas Håkansson Emulsion formation by homogenization: Current understanding and future perspectives, Annu. Rev. Food Sci. Technol., Volume 10 (2019), pp. 239-258 | DOI

[2] Nigar Kantarci; Fahir Borak; Kutlu O. Ulgen Bubble column reactors, Process Biochem., Volume 40 (2005) no. 7, pp. 2263-2283 | DOI

[3] Lu Han; Muthanna H. Al-Dahhan Gas–liquid mass transfer in a high pressure bubble column reactor with different sparger designs, Chem. Eng. Sci., Volume 62 (2007) no. 1–2, pp. 131-139 | DOI

[4] Frédéric Risso Agitation, mixing, and transfers induced by bubbles, Ann. Rev. Fluid Mech., Volume 50 (2018), pp. 25-48 | DOI | Zbl

[5] Jake J. Beaulieu; William D. Shuster; Jacob A. Rebholz Controls on gas transfer velocities in a large river, J. Geophys. Res. Biogeosci., Volume 117 (2012) no. G2, G02007, 13 pages | DOI

[6] B. O. L. Demars; J. R. Manson Temperature dependence of stream aeration coefficients and the effect of water turbulence: A critical review, Water Res., Volume 47 (2013) no. 1, pp. 1-15 | DOI

[7] W. Kendall Melville The role of surface-wave breaking in air-sea interaction, Ann. Rev. Fluid Mech., Volume 28 (1996) no. 1, pp. 279-321 | DOI

[8] D. K. Woolf; I. S. Leifer; P. D. Nightingale; T. S. Rhee; P. Bowyer; Guillemette Caulliez; G. De Leeuw; Søren Ejling Larsen; M. Liddicoat; J. Baker; M. O. Andreae Modelling of bubble-mediated gas transfer: Fundamental principles and a laboratory test, J. Marine Syst., Volume 66 (2007) no. 1–4, pp. 71-91 | DOI

[9] Luc Deike Mass transfer at the ocean–atmosphere interface: the role of wave breaking, droplets, and bubbles, Ann. Rev. Fluid Mech., Volume 54 (2022), pp. 191-224 | DOI | Zbl

[10] Nadina Müller-Fischer; Philip Tobler; Marco Dressler; Peter Fischer; Erich J. Windhab Single bubble deformation and breakup in simple shear flow, Exp. Fluids, Volume 45 (2008), pp. 917-926 | DOI

[11] Pengbo Chu; James Finch; Ghislain Bournival; Seher Ata; Christopher Hamlett; Robert J. Pugh A review of bubble break-up, Adv. Colloid Interface Sci., Volume 270 (2019), pp. 108-122

[12] Majid Rodgar; Hélène Scolan; Jean-Louis Marié; Delphine Doppler; Jean-Philippe Matas Bubble breakup and effects of soluble surfactants on bubble dynamics in a solid-body rotating flow, Phys. Rev. Fluids, Volume 8 (2023) no. 7, 073604, 20 pages | DOI

[13] Aliénor Rivière; Laurent Duchemin; Christophe Josserand; Stéphane Perrard Bubble breakup reduced to a one-dimensional nonlinear oscillator, Phys. Rev. Fluids, Volume 8 (2023) no. 9, 094004, 12 pages | DOI

[14] Marco Crialesi-Esposito; Sergio Chibbaro; Luca Brandt The interaction of droplet dynamics and turbulence cascade, Commun. Phys., Volume 6 (2023) no. 1, 5

[15] Andrey Nikolaevich Kolmogorov On the breakage of drops in a turbulent flow, Dokl. Akad. Nauk SSSR, Volume 66 (1949), pp. 825-828 | Zbl

[16] J. O. Hinze Fundamentals of the hydrodynamic mechanism of splitting in dispersion processes, AIChE J., Volume 1 (1955) no. 3, pp. 289-295 | DOI

[17] Andrey Nikolaevich Kolmogorov The local structure of turbulence in incompressible viscous fluid for very large Reynolds’ numbers, Dokl. Akad. Nauk SSSR, Volume 30 (1941), pp. 301-305 | Zbl

[18] Alberto Vela-Martín; Marc Avila Memoryless drop breakup in turbulence, Sci. Adv., Volume 8 (2022) no. 50, eabp9561, 6 pages

[19] Rui Ni Deformation and breakup of bubbles and drops in turbulence, Ann. Rev. Fluid Mech., Volume 56 (2023), pp. 319-347 | DOI | Zbl

[20] Aliénor Rivière; Kamel Abahri; Stéphane Perrard Bubble shape oscillations in a turbulent environment, J. Fluid Mech., Volume 1001 (2024), A26 | DOI | Zbl | MR

[21] Frédéric Risso; Jean Fabre Oscillations and breakup of a bubble immersed in a turbulent field, J. Fluid Mech., Volume 372 (1998), pp. 323-355 | DOI | Zbl

[22] Sophie Galinat; Frédéric Risso; Olivier Masbernat; Pascal Guiraud Dynamics of drop breakup in inhomogeneous turbulence at various volume fractions, J. Fluid Mech., Volume 578 (2007), pp. 85-94 | DOI | Zbl

[23] Benjamin Lalanne; Olivier Masbernat; Frédéric Risso A model for drop and bubble breakup frequency based on turbulence spectra, AIChE J., Volume 65 (2019) no. 1, pp. 347-359 | DOI

[24] Ashik Ullah Mohammad Masuk; Ashwanth KR Salibindla; Rui Ni Simultaneous measurements of deforming Hinze-scale bubbles with surrounding turbulence, J. Fluid Mech., Volume 910 (2021), A21, 25 pages | DOI | Zbl | MR

[25] Ignacio Roa; Marie-Charlotte Renoult; Christophe Dumouchel; Jorge César Brändle de Motta Droplet oscillations in a turbulent flow, Front. Phys., Volume 11 (2023), 1173521, 12 pages | DOI

[26] John William Strutt On the capillary phenomena of jets, Proc. R. Soc. Lond., Volume 29 (1879) no. 196–199, pp. 71-97 | DOI

[27] Horace Lamb Hydrodynamics, Cambridge University Press, 1932 | MR

[28] Florent Ravelet; Catherine Colin; Frédéric Risso On the dynamics and breakup of a bubble rising in a turbulent flow, Phys. Fluids, Volume 23 (2011) no. 10, 103301 | Zbl | DOI

[29] Stéphane Perrard; Aliénor Rivière; Wouter Mostert; Luc Deike Bubble deformation by a turbulent flow, J. Fluid Mech., Volume 920 (2021), A15 | DOI | MR

[30] S. R. Berry; Robert W. Hyers; L. M. Racz; B. Abedian Surface oscillations of an electromagnetically levitated droplet, Int. J. Thermophys., Volume 26 (2005), pp. 1565-1581 | DOI

[31] Xiao Xiao; Jürgen Brillo; Jonghyun Lee; Robert W. Hyers; Douglas M Matson Impact of convection on the damping of an oscillating droplet during viscosity measurement using the ISS-EML facility, npj Microgravity, Volume 7 (2021) no. 1, 36, 7 pages

[32] Christophe Brouzet; Raphaël Guiné; Marie-Julie Dalbe; Benjamin Favier; Nicolas Vandenberghe; Emmanuel Villermaux; Gautier Verhille Laboratory model for plastic fragmentation in the turbulent ocean, Phys. Rev. Fluids, Volume 6 (2021) no. 2, 024601, 23 pages

[33] C. A. Coulaloglou; Lawrence L. Tavlarides Description of interaction processes in agitated liquid-liquid dispersions, Chem. Eng. Sci., Volume 32 (1977) no. 11, pp. 1289-1297 | DOI

[34] Carlos Martínez-Bazán; J. L. Montanes; Juan C. Lasheras On the breakup of an air bubble injected into a fully developed turbulent flow. Part 1. Breakup frequency, J. Fluid Mech., Volume 401 (1999), pp. 157-182 | DOI

[35] Jannike Solsvik; Hugo A. Jakobsen Single air bubble breakup experiments in stirred water tank, Int. J. Chem. Reactor Eng., Volume 13 (2015) no. 4, pp. 477-491 | DOI

[36] Jiří Vejražka; Mária Zedníková; Petr Stanovskỳ Experiments on breakup of bubbles in a turbulent flow, AIChE J., Volume 64 (2018) no. 2, pp. 740-757 | DOI

[37] Aliénor Rivière; Wouter Mostert; Stéphane Perrard; Luc Deike Sub-Hinze scale bubble production in turbulent bubble break-up, J. Fluid Mech., Volume 917 (2021), A40 | DOI | MR

[38] Shijie Zhong; Rui Ni On the breakup frequency of bubbles and droplets in turbulence: a compilation and evaluation of experimental data, Int. J. Multiphase Flow, Volume 176 (2024), 104842

[39] Andreas Håkansson On the validity of different methods to estimate breakup frequency from single drop experiments, Chem. Eng. Sci., Volume 227 (2020), 115908

[40] Aliénor Rivière; Daniel J. Ruth; Wouter Mostert; Luc Deike; Stéphane Perrard Capillary driven fragmentation of large gas bubbles in turbulence, Phys. Rev. Fluids, Volume 7 (2022) no. 8, 083602, 11 pages | DOI

[41] Daniel D. Joseph Cavitation and the state of stress in a flowing liquid, J. Fluid Mech., Volume 366 (1998), pp. 367-378 | DOI

[42] Kenneth T. Kiger; James H. Duncan Air-entrainment mechanisms in plunging jets and breaking waves, Ann. Rev. Fluid Mech., Volume 44 (2012), pp. 563-596 | DOI

[43] Grant B. Deane; M. Dale Stokes Scale dependence of bubble creation mechanisms in breaking waves, Nature, Volume 418 (2002) no. 6900, pp. 839-844 | DOI

Cited by Sources:

Comments - Policy