History and future of the molecular spectroscopic databases

Laurence S. Rothman; Nicole Jacquinet-Husson; Christian Boulet; Agnès M. Perrin

doi:10.1016/j.crhy.2005.09.001

Spectroscopy and planetary atmospheres/Spectroscopie et atmosphères planétaires

History and future of the molecular spectroscopic databases
[Histoire et avenir des banques de données spectroscopiques moléculaires]

Laurence S. Rothman ¹ ; Nicole Jacquinet-Husson ² ; Christian Boulet ^3,⁴ ; Agnès M. Perrin ³

¹ Harvard-Smithsonian Center for Astrophysics, Atomic and Molecular Physics Division, 60 Garden St, Cambridge MA 02138, USA
² École polytechnique, laboratoire de météorologie dynamique, 91128 Palaiseau, France
³ Universités Paris 12 et 7, laboratoire interuniversitaire de systèmes atmosphériques (LISA), 61, avenue du Général de Gaulle, 94010 Créteil, France
⁴ Laboratoire de photophysique moléculaire, CNRS, université Paris-sud, 91405 Orsay, France

Comptes Rendus. Physique, Volume 6 (2005) no. 8, pp. 897-907.

Résumé
Abstract

On présente tout d'abord un bref historique et une revue du développement de quelques banques de données spectroscopiques moléculaires. Il s'agit de compilations des paramètres spectroscopiques nécessaires au calcul du coefficient d'absorption des espèces moléculaires que l'on rencontre dans les codes de transferts radiatifs. Le sondage de l'atmosphère terrestre a, par ailleurs, beaucoup progressé dans les dernières années, avec comme conséquence une demande accrue aux banques de données d'étendre leur couverture, aussi bien en termes d'espèces moléculaires, de domaine spectral mais aussi de précision. On présente dans cet article, quelques problèmes d'actualité illustrant diverses lacunes des banques actuelles (positions des raies, intensités, profils spectraux, …) ainsi que quelques pistes d'évolutions futures.

A brief history and review of the development of some molecular spectroscopic databases is presented. Such databases are compilations of spectroscopic parameters whose principal purpose is to provide the necessary molecular absorption input for transmission and radiance codes. Remote sensing of the terrestrial atmosphere has advanced significantly in recent years, and this has placed greater demands on the compilations in terms of accuracy, additional species, and spectral coverage. This paper discusses current pressing issues, such as the deficiencies in line positions, intensities, and line shape, as well as the directions of future enhancements.

Publié le : 2005-10-01

DOI : 10.1016/j.crhy.2005.09.001

Keywords: Spectroscopic database, Molecular spectroscopy, Line shape, Absorption parameters, Infrared cross-sections, HITRAN, GEISA, MIPAS
Mot clés : Banques de données spectroscopiques, Spectroscopie moléculaire, Profil spectral, Paramètres d'absorption, Sections efficaces (infrarouge), HITRAN, GEISA, MIPAS

Affiliations des auteurs :

Laurence S. Rothman ¹ ; Nicole Jacquinet-Husson ² ; Christian Boulet ^{3, 4} ; Agnès M. Perrin ³

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Laurence S. Rothman; Nicole Jacquinet-Husson; Christian Boulet; Agnès M. Perrin. History and future of the molecular spectroscopic databases. Comptes Rendus. Physique, Volume 6 (2005) no. 8, pp. 897-907. doi : 10.1016/j.crhy.2005.09.001. https://comptes-rendus.academie-sciences.fr/physique/articles/10.1016/j.crhy.2005.09.001/

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