[Cellules solaires à hétérojonction à base de nanofils de TiO2 et de P3HT]
Depuis plus de deux décennies, les cellules solaires organiques basées sur l'utilisation de molécules ou de polymères semi-conducteurs ont démontré de fortes potentialités. Néanmoins, et pour répondre aux limitations intrinsèques dues aux matériaux organiques (nature de l'exciton, durée de vie limitée, etc.), de nouvelles stratégies de composants hybrides basés sur l'association de matériaux organiques et inorganiques ont vu le jour. Ces nouvelles approches, basées sur l'utilisation de couches mésoporeuses inorganiques ou de nanocristaux semi-conducteurs accepteurs d'électrons, permettent en particulier un contrôle fin des architectures et des interfaces à l'échelle nanométrique. Dans ce contexte, ce travail a pour objectif la description des potentialités des composants hybrides pour la conversion photovoltaïque en s'appuyant sur un exemple récent de cellule à hétérojonction basée sur le mélange de nanofils de TiO2 avec un polymère conjugué.
Over the past decades, organic solar cells based on semiconducting polymers or small molecules have become a promising alternative to traditional inorganic photovoltaic devices. However, to address the intrinsic limitations of organic materials, such as charge separation yield, charge transport and durability, new strategies based on hybrid organic/inorganic materials have been explored. One such approach exploits mesoporous inorganic nanostructures as electron acceptors, which takes advantage of the potential to control the active layer structure and interface morphology through nanoparticle synthesis and processing. In this work, the potential of hybrid photovoltaics will be discussed and illustrated through a recent study of bulk heterojunction systems based on the blend of TiO2 nanorods with a conjugated polymer.
Mots-clés : Cellules solaires à heterojunction, Composants hybrides, Polymère conjugués, P3HT, Nanocristaux semi-conducteurs, TiO2
Johann Bouclé 1, 2 ; Sabina Chyla 3 ; Milo S.P. Shaffer 3 ; James R. Durrant 3 ; Donal D.C. Bradley 1 ; Jenny Nelson 1
@article{CRPHYS_2008__9_1_110_0,
author = {Johann Boucl\'e and Sabina Chyla and Milo S.P. Shaffer and James R. Durrant and Donal D.C. Bradley and Jenny Nelson},
title = {Hybrid bulk heterojunction solar cells based on blends of {TiO\protect\textsubscript{2}} nanorods and {P3HT}},
journal = {Comptes Rendus. Physique},
pages = {110--118},
publisher = {Elsevier},
volume = {9},
number = {1},
year = {2008},
doi = {10.1016/j.crhy.2007.10.005},
language = {en},
}
TY - JOUR AU - Johann Bouclé AU - Sabina Chyla AU - Milo S.P. Shaffer AU - James R. Durrant AU - Donal D.C. Bradley AU - Jenny Nelson TI - Hybrid bulk heterojunction solar cells based on blends of TiO2 nanorods and P3HT JO - Comptes Rendus. Physique PY - 2008 SP - 110 EP - 118 VL - 9 IS - 1 PB - Elsevier DO - 10.1016/j.crhy.2007.10.005 LA - en ID - CRPHYS_2008__9_1_110_0 ER -
%0 Journal Article %A Johann Bouclé %A Sabina Chyla %A Milo S.P. Shaffer %A James R. Durrant %A Donal D.C. Bradley %A Jenny Nelson %T Hybrid bulk heterojunction solar cells based on blends of TiO2 nanorods and P3HT %J Comptes Rendus. Physique %D 2008 %P 110-118 %V 9 %N 1 %I Elsevier %R 10.1016/j.crhy.2007.10.005 %G en %F CRPHYS_2008__9_1_110_0
Johann Bouclé; Sabina Chyla; Milo S.P. Shaffer; James R. Durrant; Donal D.C. Bradley; Jenny Nelson. Hybrid bulk heterojunction solar cells based on blends of TiO2 nanorods and P3HT. Comptes Rendus. Physique, New concepts for nanophotonics and nano-electronics, Volume 9 (2008) no. 1, pp. 110-118. doi : 10.1016/j.crhy.2007.10.005. https://comptes-rendus.academie-sciences.fr/physique/articles/10.1016/j.crhy.2007.10.005/
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