Carbon nanotube chemistry and assembly for electronic devices

Vincent Derycke; Stéphane Auvray; Julien Borghetti; Chia-Ling Chung; Roland Lefèvre; Alejandro Lopez-Bezanilla; Khoa Nguyen; Gaël Robert; Gregory Schmidt; Costin Anghel; Nicolas Chimot; Sébastien Lyonnais; Stéphane Streiff; Stéphane Campidelli; Pascale Chenevier; Arianna Filoramo; Marcelo F. Goffman; Laurence Goux-Capes; Sylvain Latil; Xavier Blase; François Triozon; Stephan Roche; Jean-Philippe Bourgoin

doi:10.1016/j.crhy.2009.05.006

Carbon nanotube chemistry and assembly for electronic devices
[Fonctionnalisation chimique et assemblage des nanotubes de carbone pour l'électronique]

Vincent Derycke ¹ ; Stéphane Auvray ¹ ; Julien Borghetti ¹ ; Chia-Ling Chung ¹ ; Roland Lefèvre ¹ ; Alejandro Lopez-Bezanilla ² ; Khoa Nguyen ¹ ; Gaël Robert ¹ ; Gregory Schmidt ¹ ; Costin Anghel ¹ ; Nicolas Chimot ¹ ; Sébastien Lyonnais ¹ ; Stéphane Streiff ¹ ; Stéphane Campidelli ¹ ; Pascale Chenevier ¹ ; Arianna Filoramo ¹ ; Marcelo F. Goffman ¹ ; Laurence Goux-Capes ¹ ; Sylvain Latil ³ ; Xavier Blase ⁴ ; François Triozon ⁵ ; Stephan Roche ² ; Jean-Philippe Bourgoin ¹

¹ Laboratoire d'Électronique Moléculaire, Service de Physique de l'État Condensé (CNRS URA 2464), CEA, IRAMIS, 91191 Gif-sur-Yvette, France
² SPSMS, CEA, INAC, 17, avenue des Martyrs, 38054 Grenoble, France
³ Service de Physique et Chimie des Surfaces et Interfaces, CEA, IRAMIS, 91191 Gif-sur-Yvette, France
⁴ Institut Néel, CNRS and université Joseph-Fourier, BP 166, 38042 Grenoble cedex 9, France
⁵ CEA, LETI, MINATEC, 38054 Grenoble, France

Comptes Rendus. Physique, Carbon nanotube electronics, Volume 10 (2009) no. 4, pp. 330-347.

Résumé
Abstract

Les nanotubes de carbone (CNTs) ont des propriétés physiques exceptionnelles qui en font l'une des briques de base les plus prometteuses des nanotechnologies. En particulier, ils peuvent jouer un rôle important pour le développement de composants électroniques innovants dans les domaines de l'électronique flexible, des détecteurs ultra-sensibles, de l'électronique haute fréquence, de l'optoélectronique, des sources d'énergie et des systèmes nano-électromécaniques (NEMS). Des démonstrations de faisabilité ont été réalisées, souvent à l'échelle du composant individuel, mais il reste de nombreux verrous à lever avant que ne puisse être évaluée la viabilité de ces composants. Le contrôle de la synthèse et celui du positionnement sont notamment critiques. Nous pensons que l'utilisation réellement innovante de ces nano-objets peut venir de (i) la combinaison de plusieurs de leurs propriétés (électriques et mécaniques par exemple) ; (ii) la combinaison de leurs propriétés avec les bénéfices additionnels apportés par d'autres molécules greffées sur les nanotubes (cette voie est particulièrement pertinente pour les détecteurs de gaz, les détecteurs de molécules biologiques, l'optoélectronique et les sources d'énergie) ; et (iii) l'utilisation de méthodes d'auto-assemblage chimiques ou bio-dirigées permettant de combiner les dispositifs en circuits. Dans cet article, nous présentons une revue de nos travaux récents concernant la chimie et l'assemblage des nanotubes et leur utilisation pour le développement de dispositifs électroniques. En particulier, nous présentons des transistors à nanotubes de carbone et leur optimisation par voie chimique, des transistors haute fréquence, des composants optoélectroniques fonctionnant comme des mémoires et des composants nano-électromécaniques. L'impact de la fonctionnalisation chimique sur les propriétés électroniques des CNTs est analysé sur la base d'études théoriques.

Carbon nanotubes (CNTs) have exceptional physical properties that make them one of the most promising building blocks for future nanotechnologies. They may in particular play an important role in the development of innovative electronic devices in the fields of flexible electronics, ultra-high sensitivity sensors, high frequency electronics, opto-electronics, energy sources and nano-electromechanical systems (NEMS). Proofs of concept of several high performance devices already exist, usually at the single device level, but there remain many serious scientific issues to be solved before the viability of such routes can be evaluated. In particular, the main concern regards the controlled synthesis and positioning of nanotubes. In our opinion, truly innovative use of these nano-objects will come from: (i) the combination of some of their complementary physical properties, such as combining their electrical and mechanical properties; (ii) the combination of their properties with additional benefits coming from other molecules grafted on the nanotubes (this route being particularly relevant for gas- and bio-sensors, opto-electronic devices and energy sources); and (iii) the use of chemically- or bio-directed self-assembly processes to allow the efficient combination of several devices into functional arrays or circuits. In this article, we review our recent results concerning nanotube chemistry and assembly and their use to develop electronic devices. In particular, we present carbon nanotube field effect transistors and their chemical optimization, high frequency nanotube transistors, nanotube-based opto-electronic devices with memory capabilities and nanotube-based nano-electromechanical systems (NEMS). The impact of chemical functionalization on the electronic properties of CNTs is analyzed on the basis of theoretical calculations.

Publié le : 2009-05-01

DOI : 10.1016/j.crhy.2009.05.006

Keywords: Carbon nanotubes, Functionalization, Self-assembly, Transistors, CNTFET, NEMS
Mots-clés : Nanotubes de carbone, Fonctionnalisation, Auto-assemblage, Transistors, CNTFET, NEMS

Affiliations des auteurs :

Vincent Derycke ¹ ; Stéphane Auvray ¹ ; Julien Borghetti ¹ ; Chia-Ling Chung ¹ ; Roland Lefèvre ¹ ; Alejandro Lopez-Bezanilla ² ; Khoa Nguyen ¹ ; Gaël Robert ¹ ; Gregory Schmidt ¹ ; Costin Anghel ¹ ; Nicolas Chimot ¹ ; Sébastien Lyonnais ¹ ; Stéphane Streiff ¹ ; Stéphane Campidelli ¹ ; Pascale Chenevier ¹ ; Arianna Filoramo ¹ ; Marcelo F. Goffman ¹ ; Laurence Goux-Capes ¹ ; Sylvain Latil ³ ; Xavier Blase ⁴ ; François Triozon ⁵ ; Stephan Roche ² ; Jean-Philippe Bourgoin ¹

¹ Laboratoire d'Électronique Moléculaire, Service de Physique de l'État Condensé (CNRS URA 2464), CEA, IRAMIS, 91191 Gif-sur-Yvette, France
² SPSMS, CEA, INAC, 17, avenue des Martyrs, 38054 Grenoble, France
³ Service de Physique et Chimie des Surfaces et Interfaces, CEA, IRAMIS, 91191 Gif-sur-Yvette, France
⁴ Institut Néel, CNRS and université Joseph-Fourier, BP 166, 38042 Grenoble cedex 9, France
⁵ CEA, LETI, MINATEC, 38054 Grenoble, France

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     author = {Vincent Derycke and St\'ephane Auvray and Julien Borghetti and Chia-Ling Chung and Roland Lef\`evre and Alejandro Lopez-Bezanilla and Khoa Nguyen and Ga\"el Robert and Gregory Schmidt and Costin Anghel and Nicolas Chimot and S\'ebastien Lyonnais and St\'ephane Streiff and St\'ephane Campidelli and Pascale Chenevier and Arianna Filoramo and Marcelo F. Goffman and Laurence Goux-Capes and Sylvain Latil and Xavier Blase and Fran\c{c}ois Triozon and Stephan Roche and Jean-Philippe Bourgoin},
     title = {Carbon nanotube chemistry and assembly for electronic devices},
     journal = {Comptes Rendus. Physique},
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     volume = {10},
     number = {4},
     year = {2009},
     doi = {10.1016/j.crhy.2009.05.006},
     language = {en},
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AU  - Nicolas Chimot
AU  - Sébastien Lyonnais
AU  - Stéphane Streiff
AU  - Stéphane Campidelli
AU  - Pascale Chenevier
AU  - Arianna Filoramo
AU  - Marcelo F. Goffman
AU  - Laurence Goux-Capes
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AU  - François Triozon
AU  - Stephan Roche
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%A Pascale Chenevier
%A Arianna Filoramo
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%A Xavier Blase
%A François Triozon
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Vincent Derycke; Stéphane Auvray; Julien Borghetti; Chia-Ling Chung; Roland Lefèvre; Alejandro Lopez-Bezanilla; Khoa Nguyen; Gaël Robert; Gregory Schmidt; Costin Anghel; Nicolas Chimot; Sébastien Lyonnais; Stéphane Streiff; Stéphane Campidelli; Pascale Chenevier; Arianna Filoramo; Marcelo F. Goffman; Laurence Goux-Capes; Sylvain Latil; Xavier Blase; François Triozon; Stephan Roche; Jean-Philippe Bourgoin. Carbon nanotube chemistry and assembly for electronic devices. Comptes Rendus. Physique, Carbon nanotube electronics, Volume 10 (2009) no. 4, pp. 330-347. doi : 10.1016/j.crhy.2009.05.006. https://comptes-rendus.academie-sciences.fr/physique/articles/10.1016/j.crhy.2009.05.006/

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