DNA – novel nanomaterial for applications in photonics and in electronics

Ileana Rau; James G. Grote; Francois Kajzar; Agnieszka Pawlicka

doi:10.1016/j.crhy.2012.09.005

Nanophotonics and near field / Nanophotonique et champ proche

DNA – novel nanomaterial for applications in photonics and in electronics
[ADN – nanomatériau nouveau pour les applications en photonique et en électronique]

Ileana Rau ¹ ; James G. Grote ² ; Francois Kajzar ^1,³ ; Agnieszka Pawlicka ⁴

¹ Faculty of Applied Chemistry and Materials Science, University Politehnica Bucharest, Bucharest, Romania
² Air Force Research Laboratory, AFRL/RXPS, 3005 Hobson Way, Wright–Patterson Air Force Base, OH 45433-7707, USA
³ Université dʼAngers, institut des sciences et technologies moleculaires dʼAngers, MOLTECH Anjou – UMR CNRS 6200, équipe interaction moleculaire optique non lineaire et structuration MINOS, 2, boulevard Lavoisier, 49045 Angers cedex, France
⁴ IQSC, Universidade de São Paulo, C.P. 780, CEP 13566-590, São Carlos, SP, Brazil

Comptes Rendus. Physique, Volume 13 (2012) no. 8, pp. 853-864.

Résumé
Abstract

Fonctionnalisation de lʼacide désoxyribonucléique (ADN) avec des composées tensioactifs et avec les molécules actives, la fabrication des films minces ainsi que leurs propriétés optiques linéaires, non linéaires et électriques sont examinées et discutées. Avec lʼaide dʼun modèle quantique à trois niveaux nous montrons que la variation anormale de la susceptibilité cubique en fonction de la concentration du chromophore dans des films minces faits à partir des complexes ADN–CTMA, dopés avec le Disperse Red 1, peut être expliquée par le déplacement de la bande dʼabsorption. Nous décrivons également comment lʼADN peut être plastifié et transformé en membranes conductrices. La conductivité électrique de ces membranes peut être contrôlée par un dopage adéquat avec des ions ou polymères conducteurs. Les membranes obtenues montrent une conductivité électrique élevée. La conductivité, mesurée à lʼambiante, varies entre de $3.5 \times 10^{- 4}$ et $10^{- 5} S / cm$ en fonction du dopant utilisé. Elle croit avec la température, pour attendre ca $10^{- 3} S / cm$ , dans le meilleur cas, à 358 K, en obéissant essentiellement la loi dʼArrhénius. Les applications pratiques des complexes dérivés de lʼADN sont également décrites et discutés.

Functionalization with surfactants and with active molecules of deoxyribonucleic acid (DNA), thin film processing as well as their nonlinear optical and electrical properties are reviewed and discussed. On the basis of a quantum three level model, we show that the anomalous concentration variation of cubic susceptibility $χ^{(3)} (- 3 ω; ω, ω, ω)$ in thin films of DNA–CTMA complexes doped with Disperse Red 1 chromophore can be explained by the concentration variation of two-photon resonance contribution. We show also that the DNA complexes, plasticized with glycerol and adequately doped can be processed into self standing conducting membranes with a high electrical conductivity. The measured ionic conductivity at room temperature, depending on dopant used and its concentration, is in the range of $3.5 \times 10^{- 4}$ – $10^{- 5} S / cm$ and increases linearly as a function of temperature, reaching $10^{- 3} S / cm$ at 358 K for the most conducting sample, obeying predominantly the Arrhenius law. Practical applications of DNA complexes are also described and discussed.

Publié le : 2012-10-01

DOI : 10.1016/j.crhy.2012.09.005

Keywords: Deoxyribonucleic acid, DNA–CTMA complex, Functionalized DNA–CTMA, NLO properties, Third harmonic generation, Solid electrochromic cells
Mot clés : Lʼacide désoxyribonucléique, LʼADN–CTMA, LʼADN–CTMA fonctionnalisé, Propriétés optiques non linéaires, De troisième génération dʼharmonique trois, Cellule électrochromique solide

Affiliations des auteurs :

Ileana Rau ¹ ; James G. Grote ² ; Francois Kajzar ^{1, 3} ; Agnieszka Pawlicka ⁴

¹ Faculty of Applied Chemistry and Materials Science, University Politehnica Bucharest, Bucharest, Romania
² Air Force Research Laboratory, AFRL/RXPS, 3005 Hobson Way, Wright–Patterson Air Force Base, OH 45433-7707, USA
³ Université dʼAngers, institut des sciences et technologies moleculaires dʼAngers, MOLTECH Anjou – UMR CNRS 6200, équipe interaction moleculaire optique non lineaire et structuration MINOS, 2, boulevard Lavoisier, 49045 Angers cedex, France
⁴ IQSC, Universidade de São Paulo, C.P. 780, CEP 13566-590, São Carlos, SP, Brazil

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Ileana Rau; James G. Grote; Francois Kajzar; Agnieszka Pawlicka. DNA – novel nanomaterial for applications in photonics and in electronics. Comptes Rendus. Physique, Volume 13 (2012) no. 8, pp. 853-864. doi : 10.1016/j.crhy.2012.09.005. https://comptes-rendus.academie-sciences.fr/physique/articles/10.1016/j.crhy.2012.09.005/

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