Precise determination of the Doppler width of a rovibrational absorption line using a comb-locked diode laser

Koichi M.T. Yamada; Atsushi Onae; Feng-Lei Hong; Hajime Inaba; Tadao Shimizu

doi:10.1016/j.crhy.2009.10.011

Precise determination of the Doppler width of a rovibrational absorption line using a comb-locked diode laser
[Détermination expérimentale de la largeur Doppler d'une raie d'absorption moléculaire rovibrationnelle en utilisant une diode laser asservie à l'aide d'un peigne de fréquences]

Koichi M.T. Yamada ¹ ; Atsushi Onae ² ; Feng-Lei Hong ² ; Hajime Inaba ² ; Tadao Shimizu ²

¹ Institute for Environmental Management Technology (EMTech), AIST, Onogawa 16-1, Tsukuba 305-8569, Japan
² National Metrology Institute of Japan (NMIJ), AIST, Umezono 1-1-1, Tsukuba 305-8563, Japan

Comptes Rendus. Physique, Experimental determination of Boltzmann's constant, Volume 10 (2009) no. 9, pp. 907-915.

Résumé
Abstract

Dans un article précédent, nous avons publié les résultats obtenus pour l'observation du profil des raies d'une transition dans l'acétylène ¹³C dans le proche infrarouge. Ce travail a été effectué en utilisant un spectrométre à diode laser accordable, la fréquence du signal étant pilotée à l'aide d'un peigne de fréquences optiques [K.M.T. Yamada et al., J. Mol. Spectrosc. 249 (2008) 95–99]. Dans le présent article nous décrivons la méthode expérimentale employée et nous approfondissons l'analyse permettant de déduire de nos résultats une détermination de la constante de Boltzmann $k_{B}$ à partir de la largeur Doppler observée. Nous discutons également les difficultés restant à surmonter pour améliorer l'exactitude de la mesure de $k_{B}$ .

We had reported in a previous paper the precision measurement of line profiles of a transition of ¹³C acetylene in the near-infrared region, employing a tunable diode-laser spectrometer, the frequency of which is locked to an optical-comb signal [K.M.T. Yamada et al., J. Mol. Spectrosc. 249 (2008) 95–99]. In the present article we review the methodology for the experiment and the analysis in determining the Boltzmann constant from the Doppler width of a rovibrational transition on the basis of our experiences. Problems to be surmounted for further improvement in accuracy are discussed.

Publié le : 2009-11-01

DOI : 10.1016/j.crhy.2009.10.011

Keywords: Boltzmann constant, Doppler width, Acetylene, Frequency comb, NIR
Mots-clés : Constante de Boltzmann, Largeur Doppler, Spectroscopie IR, Peigne de frequences, Acétylène

Affiliations des auteurs :

Koichi M.T. Yamada ¹ ; Atsushi Onae ² ; Feng-Lei Hong ² ; Hajime Inaba ² ; Tadao Shimizu ²

¹ Institute for Environmental Management Technology (EMTech), AIST, Onogawa 16-1, Tsukuba 305-8569, Japan
² National Metrology Institute of Japan (NMIJ), AIST, Umezono 1-1-1, Tsukuba 305-8563, Japan

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     author = {Koichi M.T. Yamada and Atsushi Onae and Feng-Lei Hong and Hajime Inaba and Tadao Shimizu},
     title = {Precise determination of the {Doppler} width of a rovibrational absorption line using a comb-locked diode laser},
     journal = {Comptes Rendus. Physique},
     pages = {907--915},
     publisher = {Elsevier},
     volume = {10},
     number = {9},
     year = {2009},
     doi = {10.1016/j.crhy.2009.10.011},
     language = {en},
}

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Koichi M.T. Yamada; Atsushi Onae; Feng-Lei Hong; Hajime Inaba; Tadao Shimizu. Precise determination of the Doppler width of a rovibrational absorption line using a comb-locked diode laser. Comptes Rendus. Physique, Experimental determination of Boltzmann's constant, Volume 10 (2009) no. 9, pp. 907-915. doi : 10.1016/j.crhy.2009.10.011. https://comptes-rendus.academie-sciences.fr/physique/articles/10.1016/j.crhy.2009.10.011/

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